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Controlling Chemoselectivity in Vinyl and Allylic C−X Bond Activation with Palladium Catalysis…

Jan 18, 2002·It has been demonstrated that the same Pd catalyst can be used to effect allylic substitution or vinylic cross-coupling reactions selectively and interchangeably on polyfunctionalized olefin building blocks despite the differences in reaction mechanism. This was achieved by altering the pKa of the conjugate acid of the allylic leaving group while keeping the vinyl …

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